期刊信息

  • 刊名: 河北师范大学学报(自然科学版)Journal of Hebei Normal University (Natural Science)
  • 主办: 河北师范大学
  • ISSN: 1000-5854
  • CN: 13-1061/N
  • 中国科技核心期刊
  • 中国期刊方阵入选期刊
  • 中国高校优秀科技期刊
  • 华北优秀期刊
  • 河北省优秀科技期刊

基于准二维钙钛矿(GA)(MA)5Pb5I16的阻变存储器光电性能研究

  • (1.河北师范大学 化学与材料科学学院,河北省能量转换材料与器件技术创新中心,薄膜太阳能电池材料与器件河北省工程研究中心,石家庄 050024;2.石家庄铁道大学材料科学与工程学院,石家庄 050043)
  • DOI: 10.13763/j.cnki.jhebnu.nse.202503007

Photoelectric Performance of Resistive Random Access Memory Based on Quasi-two-dimensional Perovskite (GA)(MA)5Pb5I16

摘要/Abstract

摘要:

以准二维(2D)钙钛矿(GA)(MA)5Pb5I16(GA=胍,MA=甲胺)为阻变介质材料,聚甲基丙烯酸甲酯(PMMA)和氧化石墨烯(GO)为插层,制备了Ag/PMMA/(GA)(MA)5Pb5I16/GO/ITO(ITO=锡掺杂氧化铟)阻变存储器.研究结果表明,加入PMMA和GO插层的Ag/PMMA/(GA)(MA)5Pb5I16/GO/ITO器件在亮态条件下的开关比达到1 000,较暗态开关比增大了约100倍,表现出优异的光电调控性能.

Abstract:

The Ag/PMMA/(GA)(MA)5Pb5I16/GO/ITO(ITO=indium tin oxide)resistive random access memory was prepared with quasi-two-dimensional(2D) perovskite (GA)(MA)5Pb5I16(GA=guanidine,MA=methylamine) as the resistive medium material,polymethyl methacrylate(PMMA) and graphene oxide(GO) as the intercalation.The results showed that the on/off ratio of Ag/PMMA/(GA)(MA)5Pb5I16/GO/ITO device is 1 000 under illumination after the modification of PMMA and GO intercalation,about 100 times higher than that in the dark state,presenting the excellent photoelectronic regulatory properties.

参考文献 31

  • [1] TAN H W,LIU G,YANG H L,et al.Light-gated Memristor with Integrated Logic and Memory Functions[J].ACS Nano,2017,11(11):11298-11305.doi:10.1021/acsnano.7b05762
  • [2] JIA C M,ZHAO X Y,LAI Y H,et al.Highly Flexible,Robust,Stable and High Efficiency Perovskite Solar Cells Enabled by van der Waals Epitaxy on Mica Substrate[J].Nano Energy,2019,60:476-484.doi:10.1016/j.nanoen.2019.03.053
  • [3] 赵晋津,张文华.徐徐展开新型钙钛矿光电材料的神秘画卷[J].无机材料学报,2023,38(9):989-990.doi:10.15541/jim20232000 ZHAO Jinjin,ZHANG Wenhua.Unfolding the Mysterious Scroll of Novel Photoelectric Perovskite Step by Step[J].Journal of Inorganic Materials,2023,38(9):989-990.
  • [4] REN S X,YANG Z,AN S L,et al.High-efficiency Photoelectric Regulation of Resistive Switching Memory in Perovskite Quantum Dots[J].Acta Physico-Chimica Sinica,2023,39(12):2301033.doi:10.3866/pku.Whxb202301033
  • [5] LIU X M,REN S X,LI Z H,et al.Flexible Transparent High-efficiency Photoelectric Perovskite Resistive Switching Memory[J].Advanced Functional Materials,2022,32(38):2202951.doi:10.1002/adfm.202202951
  • [6] ZHANG G L,XU Y Q,YANG S,et al.Robust Mica Perovskite Photoelectric Resistive Switching Memory[J].Nano Energy,2023,106:108074.doi:10.1016/j.nanoen.2022.108074
  • [7] 郭华军,安帅领,孟婕,等.卤化物钙钛矿光电阻变机理研究进展[J].无机材料学报,2023,38(9):1005-1016.doi:10.15541/jim20230132 GUO Huajun,AN Shuailing,MENG Jie,et al.Research Progress of Photoelectric Resistive Switching Mechanism of Halide Perovskite[J].Journal of Inorganic Materials,2023,38(9):1005-1016.
  • [8] ZHAO J J,WEI L Y,JIA C M,et al.Metallic Tin Substitution of Organic Lead Perovskite Films for Efficient Solar Cells[J].Journal of Materials Chemistry A,2018,6(41):20224-20232.doi:10.1039/c8ta05282d
  • [9] YANG S,XU Y X,HAO Z K,et al.Recent Advances in High-efficiency Perovskite for Medical Sensors[J].Acta Physico-Chimica Sinica,2022,39(5):2211025.doi:10.3866/pku.Whxb202211025
  • [10] ZHAO J J,KONG G L,CHEN S L,et al.Single Crystalline CH3NH3PbI3 Self-grown on FTO/TiO2 Substrate for High Efficiency Perovskite Solar Cells[J].Science Bulletin,2017,62(17):1173-1176.doi:10.1016/j.scib.2017.08.022
  • [11] WANG P,ZHAO J J,LIU J X,et al.Stabilization of Organometal Halide Perovskite Films by SnO2 Coating with Inactive Surface Hydroxyl Groups on ZnO Nanorods[J].Journal of Power Sources,2017,339:51-60.doi:10.1016/j.jpowsour.2016.11.046
  • [12] 王烨,焦忆楠,郭军霞,等.钙钛矿太阳能电池界面工程优化研究[J].无机材料学报,2023,38(11):1323-1330.doi:10.15541/jim20230169 WANG Ye,JIAO Yinan,GUO Junxia,et al.Optimization of Interfacial Engineering of Perovskite Solar Cells[J].Journal of Inorganic Materials,2023,38(11):1323-1330.
  • [13] ]LIU F J,WANG L,WANG J W,et al.2D Ruddlesden-Popper Perovskite Single Crystal Field-effect Transistors[J].Advanced Functional Materials,2020,31(1):2005662.doi:10.1002/adfm.202005662
  • [14] FU W,CHEN H,JEN A K Y.Two-dimensional Perovskites for Photovoltaics[J].Materials Today Nano,2021,14:100117.doi:10.1016/j.mtnano.2021.100117
  • [15] MA W B,ZHANG Z L,LIU Y F,et al.Highly Efficient and Stable Quasi Two-dimensional Perovskite Solar Cells via Synergistic Effect of Dual Additives[J].Journal of Colloid and Interface Science,2023,646:922-931.doi:10.1016/j.jcis.2023.05.132
  • [16] DAI Q,MIAO Y C,QI X R,et al.Two-dimensional Hybrid Perovskite Resistive Switching Memory Inherited from Photovoltaic Devices[J].Applied Physics Letters,2023,122(7):073301.doi:10.1063/5.0134502
  • [17] CHEN L J,XI J,TEKELENBURG E K,et al.Quasi-2D Lead-tin Perovskite Memory Devices Fabricated by Blade Coating[J].Small Methods,2023,8(2):2300040.doi:10.1002/smtd.202300040
  • [18] LIU B L,LAI J N,WU D F,et al.High-performance Resistive Random Access Memories Based on Two-dimensional HAPbI4 Organic-inorganic Hybrid Perovskite[J].Journal of Physical Chemistry Letters,2022,13(33):7653-7659.doi:10.1021/acs.jpclett.2c01786
  • [19] PARK Y J,LEE J S.Controlling the Grain Size of Dion-Jacobson-phase Two-dimensional Layered Perovskite for Memory Application[J].ACS Applied Materials & Interfaces,2022,14(3):4371-4377.doi:10.1021/acsami.1c20272
  • [20] SOE C M M,STOUMPOS C C,KEPENEKIAN M,et al.New Type of 2D Perovskites with Alternating Cations in the Interlayer Space,(C(NH2)3)(CH3NH3)nPbnI3n+1:Structure,Properties,and Photovoltaic Performance[J].Journal of the American Chemical Society,2017,139(45):16297-16309.doi:10.1021/jacs.7b09096
  • [21] ZHANG Y L,YANG T H,BOBBA R S,et al.Roles of Organic Ligands in Ambient Stability of Layered Halide Perovskites[J].ACS Applied Materials & Interfaces,2022,14(29):33085-33093.doi:10.1021/acsami.2c05348
  • [22] HUANG Y W,LI Y H,LIM E L,et al.Stable Layered 2D Perovskite Solar Cells with an Efficiency of over 19% via Multifunctional Interfacial Engineering[J].Journal of the American Chemical Society,2021,143(10):3911-3917.doi:10.1021/jacs.0c13087
  • [23] YANG J,YANG T H,LIU D L,et al.Stable 2D Alternating Cation Perovskite Solar Cells with Power Conversion Efficiency >19% via Solvent Engineering[J].Solar RRL,2021,5(8):2100286.doi:10.1002/solr.202100286
  • [24] SZAFRANSKI M,JAREK M.Origin of Spontaneous Polarization and Reconstructive Phase Transition in Guanidinium Iodide[J].CrystEngComm,2013,15(23):4617-4623.doi:10.1039/c3ce26979e
  • [25] HARDING A J,DOBSON K D,OGUNNAIKE B A,et al.Thermal and Structural Characterization of Methylammonium- and Formamidinium-halide Salts[J].Physica Status Solidi A,2021,218(22):2100246.doi:10.1002/pssa.202100246
  • [26] AROBI N,AMIR-AL ZUMAHI S M,IBRAHIM K,et al.A Holistic Framework Towards Understanding the Optical and Dielectric Behaviors of CH3NH3PbCl3 Perovskites/graphene Oxide Hybrid Films for Light Absorbing Active Layer[J].Journal of Solid State Chemistry,2021,298:122137.doi:10.1016/j.jssc.2021.122137
  • [27] LUO T,ZHANG Y L,XU Z,et al.Compositional Control in 2D Perovskites with Alternating Cations in the Interlayer Space for Photovoltaics with Efficiency over 18%[J].Advanced Materials,2019,31(44):1903848.doi:10.1002/adma.201903848
  • [28] DING B,DING Y,PENG J,et al.Dopant-additive Synergism Enhances Perovskite Solar Modules[J].Nature,2024,628(8007):299-305.doi:10.1038/s41586-024-07228-z
  • [29] GHASEMI M,GUO B Y,DARABI K,et al.A Multiscale Ion Diffusion Framework Sheds Light on the Diffusion-stability-hysteresis Nexus in Metal Halide Perovskites[J].Nature Materials,2023,22(3):329-337.doi:10.1038/s41563-023-01488-2
  • [30] ZHANG Y L,PARK N G.Quasi-two-dimensional Perovskite Solar Cells with Efficiency Exceeding 22%[J].ACS Energy Letters,2022,7(2):757-765.doi:10.1021/acsenergylett.1c02645
  • [31] JI S,SUN Y S,HUO X N,et al.The Synergistic Passivation Effect of Functionally Doped Povidone-iodine on Quasi-2D Perovskite Solar Cells[J].Journal of Materials Chemistry C,2023,11(21):7039-7047.doi:10.1039/d3tc00748k